研究方向
基于材料设计与制备方面的核心竞争力,从事复合材料和分子材料方面的前沿研究,具体方向如下:
1. 基于多孔分子框架材料的主客体多孔复合材料。多孔分子框架材料包括且不限于金属有机框架(MOF)和氢键有机框架(HOF)。研究主要围绕以下两个基础科学问题展开:
(1)物质在纳米限域空间(Confined Nanospace)中的状态与性质。
(2)主客体相互作用(Host-Guest Interactions),如电荷转移和能量转移
研究方向链接:https://www.researchgate.net/project/Exploring-Host-Guest-Systems-and-Their-Derivatives-Based-on-Metal-Organic-Frameworks
代表文献:
ACS Materials Lett., 2021, 3(11), 1599–1604;
Nat. Commun., 2019, 10, 1340;
J. Am. Chem. Soc., 2018, 140(19), 6130-6136;
Mater. Horiz., 2017, 4 (1), 64–71
2. 基于功能高分子材料的互穿聚合物网络(Interpenetrating Polymer Network, IPN)复合材料。功能高分子材料包括且不限于电子或离子导电聚合物、介电弹性体等,以实现先进柔性和软体技术所需的传感、驱动、储能等功能。部分研究与Stoyan Smoukov教授(伦敦玛丽皇后大学)保持长期合作。
代表文献:
ACS Energy Lett., 2017, 2 (9), 2014-2020;
Interface Focus, 2016, 6 (4), 20160026
代表性论文专著
*所有论文请参考我的ORCID: https://orcid.org/0000-0001-7587-7681。
最新研究成果:
• Ryuichi Murase, Timothy A. Hudson, Thomas S. Aldershof, Ky V. Nguyen, Jan G. Gluschke, Elise P. Kenny, Xiuwen Zhou, Tiesheng Wang, Martin P. van Koeverden, Benjamin J. Powell, Adam P. Micolich, Brendan F. Abrahams, and Deanna M. D'Alessandro*, Multi-Redox Responsive Behavior in a Mixed-Valence Semiconducting Framework Based on Bis-[1,2,5]-thiadiazolo-tetracyanoquinodimethane, Journal of the American Chemical Society, 2022, 144 (29), pp 13242–13253
文章链接:https://doi.org/10.1021/jacs.2c03794
代表性研究成果:
• Tiesheng Wang, ... Deanna M. D'Alessandro* et al., Fluorescence Enhancement through Confined Oligomerization in Nanochannels: An Anthryl Oligomer in a Metal-Organic Framework, ACS Materials Letters, 2021, 3 (11), pp 1599–1604
文章链接:https://doi.org/10.1021/acsmaterialslett.1c00332
• Tiesheng Wang#, Lijun Gao#, ... Anthony K Cheetham, Xinhe Bao, Qiang Fu*, Stoyan K. Smoukov* et al., Rational Approach to Guest Confinement inside MOF Cavities for Low-Temperature Catalysis, Nature Communications, 2019, 10, 1340 (#共同第一作者)
文章链接:https://doi.org/10.1038/s41467-019-08972-x
媒体报道:https://www.eurekalert.org/pub_releases/2019-03/qmuo-ssc032519.php
• Tiesheng Wang, ... Mary P. Ryan, Fang Xie* et al., Tuneable fluorescence enhancement of nanostructured ZnO arrays with controlled morphology, Physical Chemistry Chemical Physics, 2018, 20 (21), pp 14828-14834
文章链接:https://doi.org/10.1039/C8CP01493K
• Tiesheng Wang, ... Anthony K. Cheetham, Stoyan K. Smoukov* et al., Bottom-up Formation of Carbon-Based Structures with Multilevel Hierarchy from MOF-Guest Polyhedra, Journal of the American Chemical Society, 2018, 140 (19), pp 6130-6136
文章链接:https://doi.org/10.1021/jacs.8b02411
媒体报道:https://www.eurekalert.org/pub_releases/2018-05/qmuo-sdh051418.php
• Kara D. Fong#, Tiesheng Wang#, ... R. Vasant Kumar, Stoyan K. Smoukov*, Semi-Interpenetrating Polymer Networks for Enhanced Supercapacitor Electrodes, ACS Energy Letters, 2017, 2 (9), pp 2014–2020 (#共同第一作者)
文章链接:https://doi.org/10.1021/acsenergylett.7b00466
• Tiesheng Wang, ... Anthony K. Cheetham, Stoyan K. Smoukov*, Functional Conductive Nanomaterials via Polymerisation in Nano-Channels: PEDOT in a MOF, Materials Horizons, 2017, 4 (1), pp 64–71
文章链接:https://doi.org/10.1039/C6MH00230G
杂志正封面:https://doi.org/10.1039/C7MH90001E
• Tiesheng Wang, Meisam Farajollahi, ... John D. W. Madden, Stoyan K. Smoukov* et al., Electroactive Polymers for Sensing, Interface Focus, 2016, 6 (4), 20160026
文章链接:https://doi.org/10.1098/rsfs.2016.0026
• Tiesheng Wang, ... Mary P. Ryan, Fang Xie* et al., Broadband enhanced fluorescence using zinc-oxide nanoflower arrays, Journal of Materials Chemistry C, 2015, 3 (11), 2656-2663
文章链接:https://doi.org/10.1039/C4TC02751E